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In this study, we evaluated the spatial and temporal trends of black carbon (BC) in the Los Angeles Basin between 2012–2013 and 2016–2017. BC concentrations were measured in seven wavelengths using Aethalometers (AE33) at four sites, including central Los Angeles (CELA), Anaheim, Fontana, and Riverside. Sources of BC were quantified using the equivalent black carbon (EBC) model. Results indicate that total BC concentrations nearly doubled in colder period compared to the warm period. Source apportionment results revealed that fossil fuel combustion has higher annual contributions (ranging from 82% in Riverside to 91% in CELA) than biomass burning (ranging from 9.3% in CELA to 18.7% in Riverside) to the total BC concentrations at all sites. This trend was more clearly observed at the sites closer to major freeways, such as CELA and Anaheim. The relative contribution of fossil fuel to total BC …