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Free-space optical communication using lasers (lasercom) is a leading contender for future space-based communication systems with potential advantages over radio frequency (RF) communication systems in size, weight, and power consumption (SWaP). Key benefits are due to the shorter wavelength: additional bandwidth and narrow beam width. The narrower beam supports higher energy density for a given aperture size, so that lasercom can transmit data at the same rate with smaller SWaP as well as improve link security since the beam footprint is smaller. Lasercom is an attractive option for improving inter-satellite links (ISL) for resource-constrained CubeSats, which have emerged as a standard form of a small satellite since 1999. However, lasercom requires much more accurate pointing because of its narrower beam width. Accurate pointing is not trivial for most CubeSat platforms due to their resource constraints. A typical 3U CubeSat is 34 cm x 10 cm x 10 cm with less than 5 kg mass and about 10 W of available orbit-average power. This thesis presents pointing and tracking technologies to support lasercom on CubeSats. It covers three critical issues: (1) attitude determination and control of CubeSats, (2) relative orbit determination, and (3) development of a miniaturized fine beam pointing module. New attitude determination and control algorithms are developed, simulated, and validated with hardware in the loop demonstrations; results indicate that lasercom at data rates competitive with or better than RF is feasible on CubeSats. For attitude determination and control (ADC), this thesis develops a new attitude estimation algorithm …