作者
Andres Castellanos-Gomez, Rafael Roldán, Emmanuele Cappelluti, Michele Buscema, Francisco Guinea, Herre SJ Van Der Zant, Gary A Steele
发表日期
2013/11/13
期刊
Nano letters
卷号
13
期号
11
页码范围
5361-5366
出版商
American Chemical Society
简介
Controlling the bandstructure through local-strain engineering is an exciting avenue for tailoring optoelectronic properties of materials at the nanoscale. Atomically thin materials are particularly well-suited for this purpose because they can withstand extreme nonhomogeneous deformations before rupture. Here, we study the effect of large localized strain in the electronic bandstructure of atomically thin MoS2. Using photoluminescence imaging, we observe a strain-induced reduction of the direct bandgap and funneling of photogenerated excitons toward regions of higher strain. To understand these results, we develop a nonuniform tight-binding model to calculate the electronic properties of MoS2 nanolayers with complex and realistic local strain geometries, finding good agreement with our experimental results.
引用总数
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学术搜索中的文章
A Castellanos-Gomez, R Roldán, E Cappelluti… - Nano letters, 2013