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In this study, a flexible strain sensor with ultrahigh stretchability, outstanding sensitivity, and excellent repeatability based on conductive carbon black (CB) and nitrile butadiene rubber (NBR) was presented. Two organic solvents with three different coating time during the dissolve-coating process were investigated. The morphology and the degradation temperature of all the NBR/CB composite films were studied, and the tensile strength, elongation at break, as well as the young’s modulus and the dissipated energy for all the specimen were revealed. The strain-sensing tests indicated that the NBR/CB film possess a good sensitivity (max. gauge factor = 24.9) and an ultrahigh sensing range (max. 681% strain). The mathematic model from Simmons for predicting the sensing behavior based on the tunneling theory was further simplified, and a novel equation was proposed for predicting the relative change …