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A hybrid inversion method was developed to estimate the leaf chlorophyll content (LCC) and canopy chlorophyll content (CCC) of crops. Fifty hyperspectral vegetation indices (VIs), such as the photochemical reflectance index (PRI) and canopy chlorophyll index (CCI), were compared to identify the appropriate VIs for crop LCC and CCC inversion. The hybrid inversion models were then generated from different modelling methods, including the curve-fitting and least squares support vector regression (LS-SVR) and random forest regression (RFR) algorithms, by using simulated Compact High Resolution Imaging Spectrometer (CHRIS) datasets that were generated by a radiative transfer model. Finally, the remote-sensing mapping of a CHRIS image was completed to test the inversion accuracy. The results showed that the remote-sensing mapping of the CHRIS image yielded an accuracy of R² = 0.77 and …