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Aiming application of the high hole drift mobility in organopolysilanes, the organopolysilane-based organic layered photoreceptors for electrophotography have been developed with phthalocyanine pigments as a photo-generating material. The photoreceptor combined with titanylphthalocyanine exhibited the high sensitivity of 1.8 cm² (μJ)⁻¹ at 780 nm and fairly good stability, suggesting the possibility for practical use of organopolysilanes.