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In article number 2306166, Tomoya Higashihara, Cheng-Liang Liu, and co-workers conducted a thorough investigation of a three-component nanocomposite comprising small molecules doped polymer/carbon nanotubes for n-type thermoelectric application. Highlighting the impact of synergistic interactions among components on achieving high n-type thermoelectric performance, successful doping of both polymer and carbon nanotubes establishes an interconnected transport pathway, thereby enhancing overall thermoelectric efficiency.