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Arusha aquifers have been exploited intensively serving as the main source of domestic water supply in the city. But the quality of groundwater is not clearly documented for future planning and management. Hydrogeochemical assessment was carried out to establish groundwater quality and its spatial distribution with the aid of geostatistical techniques. Groundwater samples were collected and analyzed for major cations and anions using conventional methods of water analysis. Well lithology and geological map were considered for hydrogeological interpretation of the area. The results of piper diagram revealed Na–K–HCO₃ water type with sodium and bicarbonate ions dominating in all samples. High fluoride concentrations and general groundwater chemistry are mainly controlled by aquifer lithology than anthropogenic activities. The levels of anthropogenic pollution indicators such as nitrate, chloride …