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The composition of the atmosphere is significant to our ecosystem. Accordingly, there is a need to sense distributions of atmospheric scatterers such as aerosols and cloud droplets. There is growing interest in recovering these scattering fields in three-dimensions (3D). Even so, current atmospheric observations usually use expensive and unscalable equipment. Moreover, current analysis retrieves partial information (e.g., cloud-base altitudes, water droplet size at cloud tops) based on simplified 1D models. To advance observations and retrievals, we develop a new computational imaging approach for sensing and analyzing the atmosphere, volumetrically. Our approach comprises a ground-based network of cameras. We deployed it in conjunction with additional remote sensing equipment, including a Raman lidar and a sunphotometer, which provide initialization for algorithms and ground truth. The camera …