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High power operation in extreme fast charging significantly increases the risk of internal faults in Electric Vehicle batteries which can lead to accelerated battery failure. Early detection of these faults is crucial for battery safety and widespread deployment of fast charging. In this setting, we propose a real-time detection framework for battery voltage and thermal faults. A major challenge in battery fault detection arises from the effect of uncertainties originating from sensor inaccuracies, nominal aging, or unmodelled dynamics. Inspired by physics-based learning, we explore a detection paradigm that combines physics-based models, model-based detection observers, and data-driven learning techniques to address this challenge. Specifically, we construct the detection observers based on an experimentally identified electrochemical-thermal model, and subsequently design the observer tuning parameters following …