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Fault diagnosis under time-varying operational conditions is always the challenge in industrial systems. The chirplet transform (CT) provides an effective first-order approximation approach, but the slow operation speed and the drawback for high-order signal analysis limit its uses. Focusing on this problem, a fast nonlinear chirplet dictionary-based sparse decomposition (FNC-SD) method for nonlinear signal analysis is proposed. By replacing the time–frequency inclination parameter in the CT with a frequency bending parameter, the proposed method can track the nonstationary signals by arbitrary order polynomial law with time by an additional degree. Considering that too many parameters will slow down the operation speed, a frequency bending operator estimation algorithm is also proposed in this paper based on the calculated rotating frequency. Therefore, a laser vibrometer is needed in the experiment to …