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In this paper, we give three new constructions of binary sequences of period AN with optimal autocorrelation value or optimal autocorrelation magnitude using N × 4 interleaved sequences. Yu and Gong recently found any binary sequence of period AN with optimal autocorrelation value constructed from an almost difference set by Arasu et al. is an N × 4 interleaved sequence for which all four columns in its N × 4 array are shift equivalent up to the complement. We found that it is not necessary that four columns are shift equivalent. Instead, it could be a pair of related sequences together with their shifts as the column sequences. The first construction is to use a generalized GMW sequence of period N = 2 ^k - 1 and its modified version, the second construction is to use a twin prime sequence of length N = p(p + 2) and its modified version, and the third construction, a pair of Legendre sequences of period N = p (p odd …