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This doctoral dissertation introduces novel security frameworks to detect sensor-based threats on smart devices and applications in smart settings such as smart home, smart office, etc. First, we present a formal taxonomy and in-depth impact analysis of existing sensor-based threats to smart devices and applications based on attack characteristics, targeted components, and capabilities. Then, we design a novel context-aware intrusion detection system, 6thSense, to detect sensor-based threats in standalone smart devices (eg, smartphone, smart watch, etc.). 6thSense considers user activity-sensor co-dependence in standalone smart devices to learn the ongoing user activity contexts and builds a context-aware model to distinguish malicious sensor activities from benign user behavior. Further, we develop a platform-independent context-aware security framework, Aegis, to detect the behavior of malicious sensors and devices in a connected smart environment (eg, smart home, offices, etc.). Aegis observes the changing patterns of the states of smart sensors and devices for user activities in a smart environment and builds a contextual model to detect malicious activities considering sensor-device-user interactions and multi-platform correlation. Then, to limit unauthorized and malicious sensor and device access, we present, kratos, a multi-user multi-device-aware access control system for smart environment and devices. kratos introduces a formal policy language to understand diverse user demands in smart environment and implements a novel policy negotiation algorithm to automatically detect and resolve conflicting user demands and limit …