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The article reports the preparation of novel composites with hierarchical porosity and their evaluation as CO₂ adsorbents. An activator solution and metakaolin were used as starting mix. Activated carbon, characterized by a surface area of 528 m²/g and a bimodal porosity centered at 4.2 Å and 10 Å, was added to the starting mix to produce hybrid composites. It was in-house produced by thermo-chemical activation of olive pomace waste. H₂O₂ and egg protein were added to the mix as a facile method to produce foamed composites. Multiphase reaction–crystallization processes, characterized by one or two thermal steps, were designed to favor geopolymerization and in-situ NaX zeolite gel conversion of metakaolin. Both the thermal procedures produce composites in forms of monoliths, as needed for application in real processes. The two thermal steps process, of which the latter is hydrothermal, increases the …