Trion formation dynamics in monolayer transition metal dichalcogenides

A Singh, G Moody, K Tran, ME Scott, V Overbeck… - Physical Review B, 2016 - APS
A Singh, G Moody, K Tran, ME Scott, V Overbeck, G Berghäuser, J Schaibley, EJ Seifert…
Physical Review B, 2016APS
We report charged exciton (trion) formation dynamics in doped monolayer transition metal
dichalcogenides, specifically molybdenum diselenide (MoS e 2), using resonant two-color
pump-probe spectroscopy. When resonantly pumping the exciton transition, trions are
generated on a picosecond time scale through exciton-electron interaction. As the pump
energy is tuned from the high energy to low energy side of the inhomogeneously broadened
exciton resonance, the trion formation time increases by∼ 50%. This feature can be …
We report charged exciton (trion) formation dynamics in doped monolayer transition metal dichalcogenides, specifically molybdenum diselenide , using resonant two-color pump-probe spectroscopy. When resonantly pumping the exciton transition, trions are generated on a picosecond time scale through exciton-electron interaction. As the pump energy is tuned from the high energy to low energy side of the inhomogeneously broadened exciton resonance, the trion formation time increases by . This feature can be explained by the existence of both localized and delocalized excitons in a disordered potential and suggests the existence of an exciton mobility edge in transition metal dichalcogenides.
American Physical Society
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