… of the spin dynamics of a crystal of Vanadyl-based molecular … between spins and lattice
vibrations, namely the spin-… to be invaluable tools for providing insights into the physics of new …

… This comparative study provides the first insight into the role … the spin–lattice relaxation time
of molecular qubits, opening … , and spin dynamics for calculation of the dynamical magnetic …

… for a crystal of Vanadyl-based molecular qubits. Our results … molecules have been brought
forward as potential qubits, … Moreover, insights regarding the shape of the spin-echo envelop …

… , and electric field are the possible stimuli. Herein, we report … the spin dynamics are closely
related to specific vibration modes. It … To get deeper insights on the relaxation mechanism, we …

… The coupling of electron spin to phonons/vibrations plays … Insightful and quantitative
comparisons can be drawn between … potential energy surfaces. Thus, for the D 4h structure, there …

… study of the spin dynamics of a crystal of Vanadyl-based molecular qubits by means of first-…
been already proven invaluable tools for providing insights into the physics of new chemical …

… -based molecular qubit and reveal that the spin lifetime at … In order to obtain similar insights
into Raman-driven relaxation, … First-principles and ML approach to lattice and spin dynamics. (…

… and its electronic and nuclear spin dynamics. Moreover, we … weak spin–phonon coupling
of the low energy vibrations. (65) … for one of the two possible molecule/tensor assignments z …

… potential quantum bits (qubits) has reinvigorated the investigation of fundamental contributions
to electron spin … 1 -limited, local modes of vibration can become the dominant mechanism …

… of known vanadyl-based qubits in similar matrices. Coherent … To gain insight into the origin
of this trend, in Table S5† we … the presence of totally symmetric vibrations located at 104 cm −…