1-kHz two-dimensional coherent anti-Stokes Raman scattering (2D-CARS) for gas-phase thermometry

JD Miller, MN Slipchenko, JG Mance, S Roy… - Optics express, 2016 - opg.optica.org
JD Miller, MN Slipchenko, JG Mance, S Roy, JR Gord
Optics express, 2016opg.optica.org
Two-dimensional gas-phase coherent anti-Stokes Raman scattering (2D-CARS)
thermometry is demonstrated at 1 kHz in a heated jet. A hybrid femtosecond/picosecond
CARS configuration is used in a two-beam phase-matching arrangement with a 100-
femtosecond pump/Stokes pulse and a 107-picosecond probe pulse. The femtosecond
pulse is generated using a mode-locked oscillator and regenerative amplifier that is
synchronized to a separate picosecond oscillator and burst-mode amplifier. The CARS …
Two-dimensional gas-phase coherent anti-Stokes Raman scattering (2D-CARS) thermometry is demonstrated at 1 kHz in a heated jet. A hybrid femtosecond/picosecond CARS configuration is used in a two-beam phase-matching arrangement with a 100-femtosecond pump/Stokes pulse and a 107-picosecond probe pulse. The femtosecond pulse is generated using a mode-locked oscillator and regenerative amplifier that is synchronized to a separate picosecond oscillator and burst-mode amplifier. The CARS signal is spectrally dispersed in a custom imaging spectrometer and detected using a high-speed camera with image intensifier. 1-kHz, single-shot planar measurements at room temperature exhibit error of 2.6% and shot-to-shot variations of 2.6%. The spatial variation in measured temperature is 9.4%. 2D-CARS temperature measurements are demonstrated in a heated O_2 jet to capture the spatiotemporal evolution of the temperature field.
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