Boron-stabilized planar neutral π-radicals with well-balanced ambipolar charge-transport properties
T Kushida, S Shirai, N Ando, T Okamoto… - Journal of the …, 2017 - ACS Publications
Organic neutral π-monoradicals are promising semiconductors with balanced ambipolar
carrier-transport abilities, which arise from virtually identical spatial distribution of their singly
occupied and unoccupied molecular orbitals, SOMO (α) and SOMO (β), respectively. Herein,
we disclose a boron-stabilized triphenylmethyl radical that shows outstanding thermal
stability and resistance toward atmospheric conditions due to the substantial spin
delocalization. The radical is used to fabricate organic Mott-insulator transistors that operate …
carrier-transport abilities, which arise from virtually identical spatial distribution of their singly
occupied and unoccupied molecular orbitals, SOMO (α) and SOMO (β), respectively. Herein,
we disclose a boron-stabilized triphenylmethyl radical that shows outstanding thermal
stability and resistance toward atmospheric conditions due to the substantial spin
delocalization. The radical is used to fabricate organic Mott-insulator transistors that operate …
[引用][C] Boron-Stabilized Planar Neutral π-Radicals with Well-Balanced Ambipolar Charge-Transport Properties
K Tomokatsu, S Shusuke, A Naoki, O Toshihiro… - 2017
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