Catalytic behavior of copper–amine complex supported on mesoporous silica SBA-15 toward mono-Aza-Michael addition: role of amine groups

A Hakiki, RM Kerbadou, B Boukoussa… - Journal of Inorganic and …, 2019 - Springer
Journal of Inorganic and Organometallic Polymers and Materials, 2019Springer
This work concerns the preparation and modification of mesoporous silica SBA-15 with
different amine-copper complexes in order to study their impact on the catalytic behavior via
Aza Michael addition. Firstly, SBA-15 was prepared hydrothermally, then functionalized by
mono-, di-and tri-amine, and in the second step, copper (II) was anchored. The catalytic
activity of these solids was evaluated at room temperature under liquid-phase conditions.
Effects of catalyst nature, catalyst mass, reaction time and the starting reagents nature were …
Abstract
This work concerns the preparation and modification of mesoporous silica SBA-15 with different amine-copper complexes in order to study their impact on the catalytic behavior via Aza Michael addition. Firstly, SBA-15 was prepared hydrothermally, then functionalized by mono-, di- and tri-amine, and in the second step, copper (II) was anchored. The catalytic activity of these solids was evaluated at room temperature under liquid-phase conditions. Effects of catalyst nature, catalyst mass, reaction time and the starting reagents nature were investigated. Cu@SBA-15 (non-aminated) was shown to be efficient in the Aza Michael addition, but after its second re-use, a progressive decrease in the product yield was obtained due to copper leaching. The catalytic behavior of all prepared catalysts showed a selective reaction via the mono-Aza-Michael addition. Amongst all the catalysts, the one containing the monoamine-copper complex led to the highest yield. This catalyst was used in four consecutive cycles without significant loss of activity, which confirms its stability.
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