Creation of the maximum coherence via adiabatic passage in the four-wave mixing process of coherent anti-Stokes Raman scattering
N Pandya, G Liu, FA Narducci, J Chathanathil… - Chemical Physics …, 2020 - Elsevier
Abstract Coherent anti-Stokes Raman scattering has been broadly used as an efficient
method for molecular identification and specification, utilizing nonlinear optics response of a
medium based on inherent and unique properties of its compounds. CARS implies the four-
wave mixing process with three beams incident on the molecules and the fourth generated
in the medium as a nonlinear response. Here we present a novel method for optimizing this
response by maximizing the vibrational coherence in the target molecules. We demonstrate …
method for molecular identification and specification, utilizing nonlinear optics response of a
medium based on inherent and unique properties of its compounds. CARS implies the four-
wave mixing process with three beams incident on the molecules and the fourth generated
in the medium as a nonlinear response. Here we present a novel method for optimizing this
response by maximizing the vibrational coherence in the target molecules. We demonstrate …
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