Enhanced Photosusceptibility near for the Light-Induced Insulator-to-Metal Phase Transition in Vanadium Dioxide

DJ Hilton, RP Prasankumar, S Fourmaux, A Cavalleri… - Physical review …, 2007 - APS
We use optical-pump terahertz-probe spectroscopy to investigate the near-threshold
behavior of the photoinduced insulator-to-metal (IM) transition in vanadium dioxide thin
films. Upon approaching T ca reduction in the fluence required to drive the IM transition is
observed, consistent with a softening of the insulating state due to an increasing metallic
volume fraction (below the percolation limit). This phase coexistence facilitates the growth of
a homogeneous metallic conducting phase following superheating via photoexcitation. A …
We use optical-pump terahertz-probe spectroscopy to investigate the near-threshold behavior of the photoinduced insulator-to-metal (IM) transition in vanadium dioxide thin films. Upon approaching a reduction in the fluence required to drive the IM transition is observed, consistent with a softening of the insulating state due to an increasing metallic volume fraction (below the percolation limit). This phase coexistence facilitates the growth of a homogeneous metallic conducting phase following superheating via photoexcitation. A simple dynamic model using Bruggeman effective medium theory describes the observed initial condition sensitivity.
American Physical Society
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