Enhanced thermoelectric properties in hybrid graphene/boron nitride nanoribbons

K Yang, Y Chen, R D'Agosta, Y Xie, J Zhong… - Physical Review B …, 2012 - APS
Physical Review B—Condensed Matter and Materials Physics, 2012APS
The thermoelectric properties of hybrid graphene/boron nitride nanoribbons (BCNNRs) are
investigated using the nonequilibrium Green's function approach. We find that the
thermoelectric figure of merit (ZT) can be remarkably enhanced by periodically embedding
hexagonal BN (h-BN) into graphene nanoribbons (GNRs). Compared to pristine GNRs, the
ZT for armchair-edged BCNNRs with width index 3 p+ 2 is enhanced 10–20 times, while the
ZT of nanoribbons with other widths is enhanced by just 1.5–3 times. As for zigzag-edge …
The thermoelectric properties of hybrid graphene/boron nitride nanoribbons (BCNNRs) are investigated using the nonequilibrium Green's function approach. We find that the thermoelectric figure of merit () can be remarkably enhanced by periodically embedding hexagonal BN (-BN) into graphene nanoribbons (GNRs). Compared to pristine GNRs, the for armchair-edged BCNNRs with width index is enhanced 10–20 times, while the of nanoribbons with other widths is enhanced by just 1.5–3 times. As for zigzag-edge nanoribbons, the is enhanced 2–3 times. This improvement comes from the combined increase in the Seebeck coefficient and the reduction in the thermal conductance outweighing the decrease in the electrical conductance. In addition, the effect of the component ratio of -BN on the thermoelectric transport properties is discussed. These results qualify BCNNRs as a promising candidate for building outstanding thermoelectric devices.
American Physical Society
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