Kirigami patterning of MXene/bacterial cellulose composite paper for all‐solid‐state stretchable micro‐supercapacitor arrays

S Jiao, A Zhou, M Wu, H Hu - Advanced Science, 2019 - Wiley Online Library
S Jiao, A Zhou, M Wu, H Hu
Advanced Science, 2019Wiley Online Library
Stretchable micropower sources with high energy density and stability under repeated
tensile deformation are key components of flexible/wearable microelectronics. Herein,
through the combination of strain engineering and modulation of the interlayer spacing,
freestanding and lightweight MXene/bacterial cellulose (BC) composite papers with
excellent mechanical stability and a high electrochemical performance are first designed
and prepared via a facile all‐solution‐based paper‐making process. Following a simple …
Abstract
Stretchable micropower sources with high energy density and stability under repeated tensile deformation are key components of flexible/wearable microelectronics. Herein, through the combination of strain engineering and modulation of the interlayer spacing, freestanding and lightweight MXene/bacterial cellulose (BC) composite papers with excellent mechanical stability and a high electrochemical performance are first designed and prepared via a facile all‐solution‐based paper‐making process. Following a simple laser‐cutting kirigami patterning process, bendable, twistable, and stretchable all‐solid‐state micro‐supercapacitor arrays (MSCAs) are further fabricated. As expected, benefiting from the high‐performance MXene/BC composite electrodes and rational sectional structural design, the resulting kirigami MSCAs exhibit a high areal capacitance of 111.5 mF cm−2, and are stable upon stretching of up to 100% elongation, and in bent or twisted states. The demonstrated combination of an all‐solution‐based MXene/BC composite paper‐making method and an easily manipulated laser‐cutting kirigami patterning technique enables the fabrication of MXene‐based deformable all‐solid‐state planar MSCAs in a simple and efficient manner while achieving excellent areal performance metrics and high stretchability, making them promising micropower sources that are compatible with flexible/wearable microelectronics.
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