Low threshold lasing in cholesteric liquid crystals

B Taheri, AF Munoz, P Palffy-Muhoray… - Molecular Crystals and …, 2001 - Taylor & Francis
B Taheri, AF Munoz, P Palffy-Muhoray, R Twieg
Molecular Crystals and Liquid Crystals Science and Technology. Section …, 2001Taylor & Francis
Cholesteric liquid crystals, due to their periodic structure and large birefringence, are 1-d
photonic band-gap materials. Circularly polarized light of the same handedness as the
cholesteric structure cannot propagate in the reflection band. We have studied the effects of
this band-gap structure on the fluorescence spectrum of dyes dissolved in the cholesteric
liquid crystal, as well as on the fluorescence spectrum of the liquid crystal itself. We have
found that emission is enhanced at the band edges, and, above a certain pump threshold …
Abstract
Cholesteric liquid crystals, due to their periodic structure and large birefringence, are 1-d photonic band-gap materials. Circularly polarized light of the same handedness as the cholesteric structure cannot propagate in the reflection band. We have studied the effects of this band-gap structure on the fluorescence spectrum of dyes dissolved in the cholesteric liquid crystal, as well as on the fluorescence spectrum of the liquid crystal itself. We have found that emission is enhanced at the band edges, and, above a certain pump threshold, lasing occurs both in dye-doped and in pure liquid crystals. Extremely low lasing thresholds and high efficiencies were observed in dye-doped systems. The results suggest an active energy transfer mechanism between the LC host and the fluorescent dye molecules.
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