Multilayered PdTe₂/GaN heterostructures for visible-blind deep-ultraviolet photodetection

Y Liang, M Ma, X Zhong, C Xie, X Tong… - IEEE Electron …, 2021 - ieeexplore.ieee.org
Y Liang, M Ma, X Zhong, C Xie, X Tong, K Xing, C Wu
IEEE Electron Device Letters, 2021ieeexplore.ieee.org
Deep-ultraviolet (DUV) photodetection has garnered extensive research interest for its vital
applications in many military and civil fields. In this work, we present the synthesis of a large-
area two-dimensional (2D) PdTe 2 multilayer, which can be directly transferred onto a GaN
substrate to construct a vertical heterostructure for visible-blind DUV photodetection. Upon
265 nm light irradiation, the heterostructure displays a distinct photovoltaic behavior,
enabling it to serve as a self-driven photodetector. The important photoresponse …
Deep-ultraviolet (DUV) photodetection has garnered extensive research interest for its vital applications in many military and civil fields. In this work, we present the synthesis of a large-area two-dimensional (2D) PdTe 2 multilayer, which can be directly transferred onto a GaN substrate to construct a vertical heterostructure for visible-blind DUV photodetection. Upon 265 nm light irradiation, the heterostructure displays a distinct photovoltaic behavior, enabling it to serve as a self-driven photodetector. The important photoresponse parameters, such as I light /I dark ratio, responsivity, specific detectivity and DUV/visible (265 nm/450 nm) rejection ratio reach as high as 10 6 , 168.5 mA/W, 5.3 ×10 12 Jones, and 10 4 , respectively, at zero bias. The responsivity can be further enhanced to 254.6 mA/W by applying a small reverse bias of -1.0 V. In addition, the photodetector can function as a DUV light image sensor to reliably record an “H” pattern with a decent resolution. The present study paves a way for designing high-performance cost-effective DUV photodetectors towards practical optoelectronic applications.
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