Photoluminescence properties of green-emitting YBO3: Ce3+, Tb3+ phosphor for near UV excitation

R Sato, S Takeshita, T Isobe… - ECS Journal of Solid …, 2012 - iopscience.iop.org
R Sato, S Takeshita, T Isobe, T Sawayama, S Niikura
ECS Journal of Solid State Science and Technology, 2012iopscience.iop.org
Abstract YBO 3: Ce 3+, Tb 3+ phosphor was prepared from rare earth oxides and boric acid
by a solid state reaction. The phosphor absorbs near UV light through 4f–5d transitions of
Ce 3+, followed by broad emissions through 5d–4f transitions of Ce 3+ and sharp emissions
through 4f–4f transitions of Tb 3+. Spectroscopic investigations for samples with various Ce
3+ and Tb 3+ concentrations reveal nonradiative energy transfer from Ce 3+ to Tb 3+.
Emission color of the YBO 3: Ce 3+, Tb 3+ varies from blue (0.163, 0.019) to green (0.321 …
Abstract
YBO 3: Ce 3+, Tb 3+ phosphor was prepared from rare earth oxides and boric acid by a solid state reaction. The phosphor absorbs near UV light through 4f–5d transitions of Ce 3+, followed by broad emissions through 5d–4f transitions of Ce 3+ and sharp emissions through 4f–4f transitions of Tb 3+. Spectroscopic investigations for samples with various Ce 3+ and Tb 3+ concentrations reveal nonradiative energy transfer from Ce 3+ to Tb 3+. Emission color of the YBO 3: Ce 3+, Tb 3+ varies from blue (0.163, 0.019) to green (0.321, 0.585) depending on the Ce 3+ and Tb 3+ concentrations. The optimized green-emitting Y 0.82 Ce 0.03 Tb 0.15 BO 3 phosphor has an emission color of (0.309, 0.547) with an external quantum efficiency of 76.7%. The photoluminescence intensity of this phosphor at 150 C keeps 87% of its intensity at room temperature, showing sufficient thermal stability for white light emitting diode applications.
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