Propagation dynamics and X-pulse formation in phase-mismatched second-harmonic generation

G Valiulis, V Jukna, O Jedrkiewicz, M Clerici… - Physical Review A …, 2011 - APS
G Valiulis, V Jukna, O Jedrkiewicz, M Clerici, E Rubino, P DiTrapani
Physical Review A—Atomic, Molecular, and Optical Physics, 2011APS
This paper concerns the theoretical, numerical, and experimental study of the second-
harmonic-generation (SHG) process under conditions of phase and group-velocity mismatch
and aims to demonstrate the dimensionality transition of the SHG process caused by the
change of the fundamental wave diameter. We show that SHG from a narrow fundamental
beam leads to the spontaneous self-phase-matching process with, in addition, the
appearance of angular dispersion for the off-axis frequency components generated. The …
This paper concerns the theoretical, numerical, and experimental study of the second-harmonic-generation (SHG) process under conditions of phase and group-velocity mismatch and aims to demonstrate the dimensionality transition of the SHG process caused by the change of the fundamental wave diameter. We show that SHG from a narrow fundamental beam leads to the spontaneous self-phase-matching process with, in addition, the appearance of angular dispersion for the off-axis frequency components generated. The angular dispersion sustains the formation of the short X pulse in the second harmonic (SH) and is recognized as three-dimensional (3D) dynamics. On the contrary, the large-diameter fundamental beam reduces the number of the degrees of freedom, does not allow the generation of the angular dispersion, and maintains the so-called one-dimensional (1D) SHG dynamics, where the self-phase-matching appears just for axial components and is accompanied by the shrinking of the SH temporal bandwidth, and sustains a long SH pulse formation. The transition from long SH pulse generation typical of the 1D dynamics to the short 3D X pulse is illustrated numerically and experimentally by changing the conditions from the self-defocusing to the self-focusing regime by simply tuning the phase mismatch. The numerical and experimental verification of the analytical results are also presented.
American Physical Society
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