Recombination of ions with electrons: Absolute rate coefficients from a storage-ring experiment and from theoretical calculations

NR Badnell, K Spruck, C Krantz, O Novotný, A Becker… - Physical Review A, 2016 - APS
NR Badnell, K Spruck, C Krantz, O Novotný, A Becker, D Bernhardt, M Grieser, M Hahn…
Physical Review A, 2016APS
Experimentally measured and theoretically calculated rate coefficients for the recombination
of W 19+([Kr] 4 d 10 4 f 9) ions with free electrons (forming W 18+) are presented. At low
electron-ion collision energies, the merged-beam rate coefficient is dominated by strong,
mutually overlapping, recombination resonances as already found previously for the
neighboring charge-state ions W 18+ and W 20+. In the temperature range where W 19+ is
expected to form in a collisionally ionized plasma, the experimentally derived recombination …
Experimentally measured and theoretically calculated rate coefficients for the recombination of ) ions with free electrons (forming ) are presented. At low electron-ion collision energies, the merged-beam rate coefficient is dominated by strong, mutually overlapping, recombination resonances as already found previously for the neighboring charge-state ions and . In the temperature range where is expected to form in a collisionally ionized plasma, the experimentally derived recombination rate coefficient deviates by up to a factor of about 20 from the theoretical rate coefficient obtained from the Atomic Data and Analysis Structure database. The present calculations, which employ a Breit–Wigner redistributive partitioning of autoionizing widths for dielectronic recombination via multi-electron resonances, reproduce the experimental findings over the entire temperature range.
American Physical Society
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