The structure, properties, and dynamics of oxygen vacancies in amorphous SiO/sub 2

CJ Nicklaw, ZY Lu, DM Fleetwood… - … on Nuclear Science, 2002 - ieeexplore.ieee.org
IEEE Transactions on Nuclear Science, 2002ieeexplore.ieee.org
Analysis of a random population of oxygen vacancies in several amorphous SiO/sub
2/structures, using first-principles calculations, shows that a distribution of defect states
exists due to different local structure. The results also reveal a new structure of an E (/spl
gamma//sup 5/)', a five-fold coordinated puckered Si atom, which assists in explaining
reverse-bias switching behavior, and the subsequent reduction of E/sub/spl
gamma//'defects. The distribution of energy levels in the amorphous SiO/sub 2/energy gap is …
Analysis of a random population of oxygen vacancies in several amorphous SiO/sub 2/ structures, using first-principles calculations, shows that a distribution of defect states exists due to different local structure. The results also reveal a new structure of an E(/spl gamma//sup 5/)', a five-fold coordinated puckered Si atom, which assists in explaining reverse-bias switching behavior, and the subsequent reduction of E/sub /spl gamma//' defects. The distribution of energy levels in the amorphous SiO/sub 2/ energy gap is consistent with experimental data on both shallow and deep hole traps. The relative frequency of the occurrence for the different hole traps is determined by examining the local geometries of all the possible oxygen vacancy sites in the amorphous structures. Most oxygen vacancies in amorphous SiO/sub 2/ are found to form dimer defects upon hole capture, with the remainder almost evenly divided between "puckered" defects that allow dipole formation upon electron capture (E(/spl gamma//sup 4/)') and those that do not (E(/spl gamma//sup 5/)').
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