Upconversion emission enhancement by porous silver films with ultra-broad plasmon absorption

B Shao, Z Yang, J Li, J Yang, Y Wang, J Qiu… - Optical Materials …, 2017 - opg.optica.org
B Shao, Z Yang, J Li, J Yang, Y Wang, J Qiu, Z Song
Optical Materials Express, 2017opg.optica.org
Surface plasmon effects of Ag nanostructures are being extensively applied to enhance
upconversion (UC) luminescence properties of rare-earth-ion-doped nanoparticles.
However, the plasmonic absorption bands from various Ag nanostructures are generally
located at a visible region that cannot couple effectively with the 980 nm near infrared
excitation light, resulting in a smaller UC emission enhancement factor. In this paper, we
present a facile method to fabricate the porous Ag films with tunable and ultra-broad surface …
Abstract
Surface plasmon effects of Ag nanostructures are being extensively applied to enhance upconversion (UC) luminescence properties of rare-earth-ion-doped nanoparticles. However, the plasmonic absorption bands from various Ag nanostructures are generally located at a visible region that cannot couple effectively with the 980 nm near infrared excitation light, resulting in a smaller UC emission enhancement factor. In this paper, we present a facile method to fabricate the porous Ag films with tunable and ultra-broad surface plasmonic absorption by using a polystyrene microsphere as a hard template, and then investigate the influence of tunable surface plasmonic absorption (SPA) on the UC emission. About 10 and 60-fold UC emission enhancement of NaYF4: Yb3+, Er3+ nanoparticles was obtained on the Ag films with narrow and ultra-broad SPA ranging from 350 to 1400 nm, respectively. The UC emission increases 60 fold at the surface of porous Ag film with the ultra-broad plasmonic absorption, which is attributed to efficient coupling between the ultra-broad SPA and the 980 nm near infrared excitation light and UC emission. The results demonstrate Ag film with ultra-broad plasmonic absorption is more appropriate as a substrate for the enhancement of UC emission in comparison with the narrow plasmonic absorption Ag film.
opg.optica.org
以上显示的是最相近的搜索结果。 查看全部搜索结果

Google学术搜索按钮

example.edu/paper.pdf
搜索
获取 PDF 文件
引用
References