Absolute nonlinear optical probes of surface chirality

MJ Huttunen, M Erkintalo… - Journal of Optics A: Pure …, 2009 - iopscience.iop.org
Journal of Optics A: Pure and Applied Optics, 2009iopscience.iop.org
We propose new nonlinear optical techniques as probes of the chirality of surfaces and thin
films. The techniques are based on surface second-harmonic generation using focused
laser beams. To avoid coupling to the possible anisotropy of the sample, which can also
lead to chiral signals and is therefore a problem of traditional second-harmonic probes of
surface chirality, the optical beams are applied at normal incidence and possess azimuthal
symmetry about the direction of propagation. The handedness is obtained by using incident …
Abstract
We propose new nonlinear optical techniques as probes of the chirality of surfaces and thin films. The techniques are based on surface second-harmonic generation using focused laser beams. To avoid coupling to the possible anisotropy of the sample, which can also lead to chiral signals and is therefore a problem of traditional second-harmonic probes of surface chirality, the optical beams are applied at normal incidence and possess azimuthal symmetry about the direction of propagation. The handedness is obtained by using incident beams that are circularly polarized or appropriate superpositions of radially and azimuthally polarized higher-order modes. We model numerically four cases of different sample symmetries and demonstrate that the techniques are sensitive only to the chirality and not to the anisotropy. The techniques are therefore absolute probes of surface chirality and are naturally applicable to the microscopy of chiral properties of thin films.
iopscience.iop.org
以上显示的是最相近的搜索结果。 查看全部搜索结果