Adsorption-mediated mass streaming in a standing acoustic wave

O Weltsch, A Offner, D Liberzon, GZ Ramon - Physical review letters, 2017 - APS
Physical review letters, 2017APS
Oscillating flows can generate nonzero, time-averaged fluxes despite the velocity averaging
zero over an oscillation cycle. Here, we report such a flux, a nonlinear resultant of the
interaction between oscillating velocity and concentration fields. Specifically, we study a gas
mixture sustaining a standing acoustic wave, where an adsorbent coats the solid boundary
in contact with the gas mixture. It is found that the sound wave produces a significant, time-
averaged preferential flux of a “reactive” component that undergoes a reversible sorption …
Oscillating flows can generate nonzero, time-averaged fluxes despite the velocity averaging zero over an oscillation cycle. Here, we report such a flux, a nonlinear resultant of the interaction between oscillating velocity and concentration fields. Specifically, we study a gas mixture sustaining a standing acoustic wave, where an adsorbent coats the solid boundary in contact with the gas mixture. It is found that the sound wave produces a significant, time-averaged preferential flux of a “reactive” component that undergoes a reversible sorption process. This effect is measured experimentally for an air-water vapor mixture. An approximate model is shown to be in good agreement with the experimental observations, and further reveals the interplay between the sound-wave characteristics and the properties of the gas-solid sorbate-sorbent pair. The preferential flux generated by this mechanism may have potential in separation processes.
American Physical Society
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