[图书][B] Converting Biomass into Renewable Fuel Intermediate-Bio-oil: Elucidating Torrefaction Effect on Bio-oil Quality and Study on Bio-oil Aging Mechanism

J Meng - 2013 - search.proquest.com
2013search.proquest.com
Converting biomass into liquid transportation fuel is of great importance for a secure energy
supply. Though biomass pyrolysis offers a convenient avenue to produce a liquid fuel
intermediate-bio-oil, a significant amount of effort is still demanded to overcome the poor oil
properties towards its application as drop-in transportation fuel. These challenges include
reducing bio-oil oxygen content, water content, acidity and improving its stability during
storage and upgrading. The current research investigated the torrefaction effect on …
Abstract
Converting biomass into liquid transportation fuel is of great importance for a secure energy supply. Though biomass pyrolysis offers a convenient avenue to produce a liquid fuel intermediate-bio-oil, a significant amount of effort is still demanded to overcome the poor oil properties towards its application as drop-in transportation fuel. These challenges include reducing bio-oil oxygen content, water content, acidity and improving its stability during storage and upgrading. The current research investigated the torrefaction effect on improving bio-oil physicochemical property and stability. In this study, fluidized-bed fast-pyrolysis was performed on torrefied loblolly pine with different torrefaction severities. The results showed that torrefaction pretreatment can significantly reduce the oxygen and water content and acidity of the bio-oil as well as varying bio-oil chemical composition with concentrated pyrolytic lignin and levoglucosan. A modified cellulose pyrolysis mechanism was proposed to explain the increased levoglucosan concentration in the torrefaction-based bio-oil. With regarding to the bio-oil stability, torrefaction based bio-oil showed less physicochemical and compositional variation than that of raw bio-oil. In addition, torrefaction based bio-oil could maintain a uniform oil phase for twelve-month storage. All these effects are attributed to the structural and compositional change of torrefied wood induced by the thermal pretreatment.
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