Decoherence Window and Electron-Nuclear Cross Relaxation in the Molecular Magnet
Rabi oscillations in the V 15 single molecule magnet embedded in the surfactant (CH 3) 2
[CH 3 (CH 2) 16 CH 2] 2 N+ have been studied at different microwave powers. An intense
damping peak is observed when the Rabi frequency Ω R falls in the vicinity of the Larmor
frequency of protons ω N. The experiments are interpreted by a model showing that the
damping (or Rabi) time τ R is directly associated with decoherence caused by electron-
nuclear cross relaxation in the rotating reference frame. This decoherence induces energy …
[CH 3 (CH 2) 16 CH 2] 2 N+ have been studied at different microwave powers. An intense
damping peak is observed when the Rabi frequency Ω R falls in the vicinity of the Larmor
frequency of protons ω N. The experiments are interpreted by a model showing that the
damping (or Rabi) time τ R is directly associated with decoherence caused by electron-
nuclear cross relaxation in the rotating reference frame. This decoherence induces energy …
Decoherence window and electron-nuclear cross relaxation in the molecular magnet V 15
Rabi oscillations in the V 15 single molecule magnet embedded in the surfactant (CH 3) 2
[CH 3 (CH 2) 16CH 2] 2N+ have been studied at different microwave powers. An intense
damping peak is observed when the Rabi frequency Ω R falls in the vicinity of the Larmor
frequency of protons ω N. The experiments are interpreted by a model showing that the
damping (or Rabi) time τ R is directly associated with decoherence caused by electron-
nuclear cross relaxation in the rotating reference frame. This decoherence induces energy …
[CH 3 (CH 2) 16CH 2] 2N+ have been studied at different microwave powers. An intense
damping peak is observed when the Rabi frequency Ω R falls in the vicinity of the Larmor
frequency of protons ω N. The experiments are interpreted by a model showing that the
damping (or Rabi) time τ R is directly associated with decoherence caused by electron-
nuclear cross relaxation in the rotating reference frame. This decoherence induces energy …
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