Dihydrodipicolinate synthase is not inhibited by its substrate,(S)-aspartate beta-semialdehyde

RCJ Dobson, JA Gerrard, FG Pearce - Biochemical Journal, 2004 - portlandpress.com
Biochemical Journal, 2004portlandpress.com
DHDPS (dihydrodipicolinate synthase; EC 4.2. 1.52) is the enzyme that catalyses the first
unique step of lysine biosynthesis in plants and micro-organisms. As such, it has attracted
much attention as a target for herbicide and anti-microbial action. DHDPS has two
substrates: pyruvate and (S)-aspartate β-semialdehyde [(S)-ASA]. There are various
literature reports that suggest that high levels of (S)-ASA inhibit the enzyme [Karsten (1997)
Biochemistry 36, 1730–1739; Stahly (1969) Biochim. Biophys. Acta 191, 439–451], whereas …
DHDPS (dihydrodipicolinate synthase; EC 4.2.1.52) is the enzyme that catalyses the first unique step of lysine biosynthesis in plants and micro-organisms. As such, it has attracted much attention as a target for herbicide and anti-microbial action. DHDPS has two substrates: pyruvate and (S)-aspartate β-semialdehyde [(S)-ASA]. There are various literature reports that suggest that high levels of (S)-ASA inhibit the enzyme [Karsten (1997) Biochemistry 36, 1730–1739; Stahly (1969) Biochim. Biophys. Acta 191, 439–451], whereas others have not observed this phenomenon. We have resolved this long-running literature debate and shown unequivocally that this difference in reported behaviour can be attributed to differences in the preparation of (S)-ASA used by each researcher. DHDPS is not inhibited by its substrate; rather, the inhibition is due to an, as yet, unidentified inhibitor in preparations of the substrate generated by ozonolysis. Furthermore, we demonstrate that (R)-ASA is neither an inhibitor nor a substrate of DHDPS from Escherichia coli.
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