Effect of an external electric field on the diffusion-influenced reversible reaction of a neutral particle and a charged particle in three dimensions
SY Reigh, KJ Shin, M Tachiya - The Journal of Chemical Physics, 2008 - pubs.aip.org
… In this work, we investigate the field effect on the diffusion-influenced geminate
recombination of a neutral particle and a charged particle in 3D. The present system is a
simplification of the Onsager problem by replacing a charged reactant with a neutral one
thus avoiding the difficulty of handling the Coulomb potential but the spatial asymmetry in
3D is retained. We investigate the reversible system by introducing a generalized
nonisotropic boundary condition taking into account of the reversibility of the reaction …
recombination of a neutral particle and a charged particle in 3D. The present system is a
simplification of the Onsager problem by replacing a charged reactant with a neutral one
thus avoiding the difficulty of handling the Coulomb potential but the spatial asymmetry in
3D is retained. We investigate the reversible system by introducing a generalized
nonisotropic boundary condition taking into account of the reversibility of the reaction …
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