can correct for changes in pathlength due to sphere wall contamination. This allows for the
gas absorption coefficient to be determined continuously without needing to recalibrate the
setup. We demonstrate the technique experimentally, measuring methane gas at 1651nm.
For example, contamination covering 1.2% of the sphere wall resulted in an uncompensated
error in gas absorption coefficient of≈ 41%. With the ratiometric scheme, this error was …