Laser stimulated chemical reactions and isotope separation
NG Basov, ÉM Belenov, VA Isakov… - Soviet Journal of …, 1975 - iopscience.iop.org
NG Basov, ÉM Belenov, VA Isakov, EP Markin, AN Oraevskii, VI Romanenko…
Soviet Journal of Quantum Electronics, 1975•iopscience.iop.orgA theoretical analysis is made of an isotope separation method based on chemical reactions
stimulated by infrared laser radiation. It is shown that the anharmonicity of the molecular
vibrations has practically no effect on the isotope separation coefficient. A description is
given of an experiment in which the nitrogen isotopes were separated by the laser-
stimulated reaction N 2+ O 2→ 2NO. This reaction was stimulated in a cell containing air
which was subjected simultaneously to ruby laser radiation and to a strong Stokes …
stimulated by infrared laser radiation. It is shown that the anharmonicity of the molecular
vibrations has practically no effect on the isotope separation coefficient. A description is
given of an experiment in which the nitrogen isotopes were separated by the laser-
stimulated reaction N 2+ O 2→ 2NO. This reaction was stimulated in a cell containing air
which was subjected simultaneously to ruby laser radiation and to a strong Stokes …
Abstract
A theoretical analysis is made of an isotope separation method based on chemical reactions stimulated by infrared laser radiation. It is shown that the anharmonicity of the molecular vibrations has practically no effect on the isotope separation coefficient. A description is given of an experiment in which the nitrogen isotopes were separated by the laser-stimulated reaction N 2+ O 2→ 2NO. This reaction was stimulated in a cell containing air which was subjected simultaneously to ruby laser radiation and to a strong Stokes component generated separately by stimulated Raman scattering in liquid nitrogen.
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