Lasonolide A: structural revision and synthesis of the unnatural (−)-enantiomer
E Lee, HY Song, JW Kang, DS Kim… - Journal of the …, 2002 - ACS Publications
E Lee, HY Song, JW Kang, DS Kim, CK Jung, JM Joo
Journal of the American Chemical Society, 2002•ACS PublicationsTotal synthesis of the unnatural (−)-enantiomer of lasonolide A was achieved starting from
ethyl l-malate. The two tetrahydropyranyl fragments were prepared stereoselectively via
radical cyclization reactions of β-alkoxyacrylates. The full structure of natural lasonolide A
was determined unequivocally.
ethyl l-malate. The two tetrahydropyranyl fragments were prepared stereoselectively via
radical cyclization reactions of β-alkoxyacrylates. The full structure of natural lasonolide A
was determined unequivocally.
Total synthesis of the unnatural (−)-enantiomer of lasonolide A was achieved starting from ethyl l-malate. The two tetrahydropyranyl fragments were prepared stereoselectively via radical cyclization reactions of β-alkoxyacrylates. The full structure of natural lasonolide A was determined unequivocally.
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