Magnetic order in the pyrochlore iridates IrO ( = Y, Yb)

SM Disseler, C Dhital, A Amato, SR Giblin… - Physical Review B …, 2012 - APS
Physical Review B—Condensed Matter and Materials Physics, 2012APS
We present results from muon spin relaxation/rotation, magnetization, neutron scattering,
and transport measurements on polycrystalline samples of the pyrochlore iridates Y 2 Ir 2 O
7 (Y-227) and Yb 2 Ir 2 O 7 (Yb-227). Well-defined spontaneous oscillations of the muon
asymmetry are observed together with hysteretic behavior in magnetization below 130 K in
Yb-227, indicative of commensurate long-range magnetic order. Similar oscillations are
observed in Y-227 below 150 K; however, the onset of hysteretic magnetization at T= 190 K …
We present results from muon spin relaxation/rotation, magnetization, neutron scattering, and transport measurements on polycrystalline samples of the pyrochlore iridates YIrO (Y-227) and YbIrO (Yb-227). Well-defined spontaneous oscillations of the muon asymmetry are observed together with hysteretic behavior in magnetization below 130 K in Yb-227, indicative of commensurate long-range magnetic order. Similar oscillations are observed in Y-227 below 150 K; however, the onset of hysteretic magnetization at 190 K indicates a transition to an intermediate state lacking long-range order as observed in Nd-227. Our results also show that insulating members of the iridate family have nearly identical magnetic ground states, and that the presence of magnetic -site species does not play any significant role in altering the ground-state properties.
American Physical Society
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