Nitric oxide formation in a premixed flame with high-level plasma energy coupling

X Rao, IB Matveev, T Lee - IEEE Transactions on plasma …, 2009 - ieeexplore.ieee.org
X Rao, IB Matveev, T Lee
IEEE Transactions on plasma science, 2009ieeexplore.ieee.org
This paper presents quantitative planar laser-induced fluorescence (PLIF) imaging of nitric
oxide (NO) in a transient-arc direct-current plasmatron igniter using premixed air/fuel
mixtures. Quantitative measurements of NO are reported as a function of gas flow rate (20-
50 standard cubic feet per hour), plasma power (100-900 mA, 150-750 W), and equivalence
ratio (0.7-1.3). Images were corrected for temperature effects by using 2-D temperature field
measurements obtained with infrared thermometry and calibrated by a more accurate …
This paper presents quantitative planar laser-induced fluorescence (PLIF) imaging of nitric oxide (NO) in a transient-arc direct-current plasmatron igniter using premixed air/fuel mixtures. Quantitative measurements of NO are reported as a function of gas flow rate (20-50 standard cubic feet per hour), plasma power (100-900 mA, 150-750 W), and equivalence ratio (0.7-1.3). Images were corrected for temperature effects by using 2-D temperature field measurements obtained with infrared thermometry and calibrated by a more accurate multiline fitting technique. The signals were then quantified using an NO addition method and spectroscopic laser-induced fluorescence modeling of NO. NO PLIF images and single-point NO concentrations are presented for both plasma-discharge-only and methane/air plasma-enhanced combustion cases. NO formation occurs predominantly through N 2 (v) + O ¿ NO + N for the plasma-discharge-only case without combustion. The NO concentration for the plasma-enhanced combustion case (500-3500 ppm) was an order of magnitude less than the plasma-discharge-only case (8000-15 000 ppm) due to the reduction of plasma reactions by the methane. Experiments show the linear decay of NO from equivalence ratio 0.8-1.2 under the same flow condition and discharge current.
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