330 K to obtain the three irreducible components of the Raman tensor (Γ 1, Γ 15, and Γ 12).
Γ 12 is found negligible. Γ 1 dominates the 2TA scattering, whereas other regions of the
spectra show both Γ 1 and Γ 15 symmetries. The Γ 1 component is compared with recent
calculations of the overtones of the two-phonon density of states based on an overlap-
valence-shell model. Good agreement is obtained. Although neutron data are not available …