Seven-octave high-brightness and carrier-envelope-phase-stable light source

U Elu, L Maidment, L Vamos, F Tani, D Novoa… - Nature …, 2021 - nature.com
U Elu, L Maidment, L Vamos, F Tani, D Novoa, MH Frosz, V Badikov, D Badikov, V Petrov
Nature Photonics, 2021nature.com
High-brightness sources of coherent and few-cycle-duration light waveforms with spectral
coverage from the ultraviolet to the terahertz would offer unprecedented versatility and
opportunities for a wide range of applications from bio-chemical sensing to time-resolved
and nonlinear spectroscopy, and to attosecond light-wave electronics,. Combinations of
various sources with frequency conversion, and supercontinuum generation,,–can provide
relatively large spectral coverage, but many applications require a much broader spectral …
Abstract
High-brightness sources of coherent and few-cycle-duration light waveforms with spectral coverage from the ultraviolet to the terahertz would offer unprecedented versatility and opportunities for a wide range of applications from bio-chemical sensing to time-resolved and nonlinear spectroscopy, and to attosecond light-wave electronics,. Combinations of various sources with frequency conversion, and supercontinuum generation, , – can provide relatively large spectral coverage, but many applications require a much broader spectral range and low-jitter synchronization for time-domain measurements. Here, we present a carrier-envelope-phase (CEP)-stable light source, seeded by a mid-infrared frequency comb,, with simultaneous spectral coverage across seven optical octaves, from the ultraviolet (340 nm) into the terahertz (40,000 nm). Combining soliton self-compression and dispersive wave generation in an anti-resonant-reflection photonic-crystal fibre with intra-pulse difference frequency generation in BaGa2GeSe6, the spectral brightness is two to five orders of magnitude above that of synchrotron sources. This will enable high-dynamic-range spectroscopies and provide numerous opportunities in attosecond physics and material sciences,.
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