Soft-lock drawing of super-aligned carbon nanotube bundles for nanometre electrical contacts

Y Guo, E Shi, J Zhu, PC Shen, J Wang, Y Lin… - Nature …, 2022 - nature.com
Nature Nanotechnology, 2022nature.com
The assembly of single-walled carbon nanotubes (CNTs) into high-density horizontal arrays
is strongly desired for practical applications, but challenges remain despite myriads of
research efforts. Herein, we developed a non-destructive soft-lock drawing method to
achieve ultraclean single-walled CNT arrays with a very high degree of alignment (angle
standard deviation of~ 0.03°). These arrays contained a large portion of nanometre-sized
CNT bundles, yielding a high packing density (~ 400 µm− 1) and high current carrying …
Abstract
The assembly of single-walled carbon nanotubes (CNTs) into high-density horizontal arrays is strongly desired for practical applications, but challenges remain despite myriads of research efforts. Herein, we developed a non-destructive soft-lock drawing method to achieve ultraclean single-walled CNT arrays with a very high degree of alignment (angle standard deviation of ~0.03°). These arrays contained a large portion of nanometre-sized CNT bundles, yielding a high packing density (~400 µm−1) and high current carrying capacity (∼1.8 × 108 A cm2). This alignment strategy can be generally extended to diverse substrates or sources of raw single-walled CNTs. Significantly, the assembled CNT bundles were used as nanometre electrical contacts of high-density monolayer molybdenum disulfide (MoS2) transistors, exhibiting high current density (~38 µA µm−1), low contact resistance (~1.6 kΩ µm), excellent device-to-device uniformity and highly reduced device areas (0.06 µm2 per device), demonstrating their potential for future electronic devices and advanced integration technologies.
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