The infrared predissociation spectra of water clusters
DF Coker, RE Miller, RO Watts - The Journal of chemical physics, 1985 - pubs.aip.org
Infrared predissociation spectra of water clusters have been measured in the frequency
range 3000–3800 cm− 1 using a molecular beam–color center laser apparatus. The
transition from a spectrum resembling that of liquid water to that of the dimer is clearly seen.
Detailed theoretical analyses using normal mode theory, local mode theory, and a quantum
simulation method are used to interpret the spectrum in terms of a potential surface that
includes both intramolecular and intermolecular degrees of freedom.
range 3000–3800 cm− 1 using a molecular beam–color center laser apparatus. The
transition from a spectrum resembling that of liquid water to that of the dimer is clearly seen.
Detailed theoretical analyses using normal mode theory, local mode theory, and a quantum
simulation method are used to interpret the spectrum in terms of a potential surface that
includes both intramolecular and intermolecular degrees of freedom.
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