Theoretical calculation of line shapes and saturation effects in polarization spectroscopy
TA Reichardt, RP Lucht - The Journal of chemical physics, 1998 - pubs.aip.org
The physics of polarization spectroscopy (PS) is investigated by direct numerical integration
of the time-dependent density matrix equations. The Zeeman structure of the upper and
lower energy levels is included in a multistate formulation of the density matrix equations.
The numerical solution of the time-dependent density matrix equations enables us to
investigate the effects of strong saturation on PS signal levels and line shapes. Bath levels
not directly coupled by the laser radiation are included in the numerical modeling to …
of the time-dependent density matrix equations. The Zeeman structure of the upper and
lower energy levels is included in a multistate formulation of the density matrix equations.
The numerical solution of the time-dependent density matrix equations enables us to
investigate the effects of strong saturation on PS signal levels and line shapes. Bath levels
not directly coupled by the laser radiation are included in the numerical modeling to …
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