Time-and frequency-dependent model of time-resolved coherent anti-Stokes Raman scattering (CARS) with a picosecond-duration probe pulse
The hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (fs/ps CARS)
technique presents a promising alternative to either fs time-resolved or ps frequency-
resolved CARS in both gas-phase thermometry and condensed-phase excited-state
dynamics applications. A theoretical description of time-dependent CARS is used to
examine this recently developed probe technique, and quantitative comparisons of the full
time–frequency evolution show excellent accuracy in predicting the experimental vibrational …
technique presents a promising alternative to either fs time-resolved or ps frequency-
resolved CARS in both gas-phase thermometry and condensed-phase excited-state
dynamics applications. A theoretical description of time-dependent CARS is used to
examine this recently developed probe technique, and quantitative comparisons of the full
time–frequency evolution show excellent accuracy in predicting the experimental vibrational …
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