High strength astringent hydrogels using protein as the building block for physically cross-linked multi-network

R Xu, S Ma, P Lin, B Yu, F Zhou… - ACS applied materials & …, 2017 - ACS Publications
Integrating proteins into a hydrogel network enables its good bioactivity as an ECM
environment in biorelative applications. Although extensive studies on preparing protein …

Highly stretchable, self-healing elastomer hydrogel with universal adhesion driven by reversible cross-links and protein enhancement

K Lei, M Chen, X Wang, J Gao, J Zhang, G Li… - Journal of Materials …, 2022 - pubs.rsc.org
Engineered hydrogels with excellent mechanical properties and multi-functionality have
great potential as soft electronic skins, tissue substitutes and flexible robotic joints. However …

Conjoined-network rendered stiff and tough hydrogels from biogenic molecules

L Xu, C Wang, Y Cui, A Li, Y Qiao, D Qiu - Science advances, 2019 - science.org
Hydrogels from biological sources are expected as potential structural biomaterials, but most
of them are either soft or fragile. Here, a new strategy was developed to construct hydrogels …

Anisotropic hydrogels with a multiscale hierarchical structure exhibiting high strength and toughness for mimicking tendons

N Park, J Kim - ACS Applied Materials & Interfaces, 2021 - ACS Publications
Owing to their anisotropic and hierarchical structure, tendons exhibit an outstanding
mechanical performance despite the low polymer concentration and softness of the …

Tough, ultrastretchable and tear-resistant hydrogels enabled by linear macro-cross-linker

Z Cao, Y Wang, H Wang, C Ma, H Li, J Zheng… - Polymer …, 2019 - pubs.rsc.org
Strong, tough and tear-resistant hydrogels hold great promise for applications as load-
bearing structural biomaterials such as cartilages, tendons and ligaments. Here, we design …

Muscle-inspired double-network hydrogels with robust mechanical property, biocompatibility and ionic conductivity

L Geng, S Hu, M Cui, J Wu, A Huang, S Shi… - Carbohydrate Polymers, 2021 - Elsevier
Inspired by muscle architectures, double network hydrogels with hierarchically aligned
structures were fabricated, where cross-linked cellulose nanofiber (CNF)/chitosan hydrogel …

A facile method to fabricate anisotropic hydrogels with perfectly aligned hierarchical fibrous structures

MTI Mredha, YZ Guo, T Nonoyama… - Advanced …, 2018 - Wiley Online Library
Natural structural materials (such as tendons and ligaments) are comprised of multiscale
hierarchical architectures, with dimensions ranging from nano‐to macroscale, which are …

Multiple physical cross-linker strategy to achieve mechanically tough and reversible properties of double-network hydrogels in bulk and on surfaces

Y Zhang, B Ren, S Xie, Y Cai, T Wang… - ACS Applied Polymer …, 2019 - ACS Publications
Development of tough and adhesive hydrogels is critical for different applications, including
wound dressing, soft robotics, and wearable devices. However, achieving strong and …

Tough hydrogel with high water content and ordered fibrous structures as an artificial human ligament

S Han, Q Wu, J Zhu, J Zhang, A Chen, S Su, J Liu… - Materials …, 2023 - pubs.rsc.org
Natural biological tissues such as ligaments, due to their anisotropic across scale structure,
have high water content, while still maintaining high strength and flexibility. Hydrogels are …

Double-network physical cross-linking strategy to promote bulk mechanical and surface adhesive properties of hydrogels

L Tang, D Zhang, L Gong, Y Zhang, S Xie, B Ren… - …, 2019 - ACS Publications
Development of mechanically strong and adhesive hydrogels with self-recovery and self-
healing properties is important for many applications but has proven to be very challenging …