A common mechanism underlies the dark fraction formation and fluorescence blinking of quantum dots

N Durisic, PW Wiseman, P Grütter, CD Heyes - Acs Nano, 2009 - ACS Publications
CdSe quantum dots (QDs) are known to exhibit both power-law blinking dynamics and a
dark fraction. A complete description of the mechanistic origins of these properties is still …

Shell-dependent photoluminescence studies provide mechanistic insights into the off–grey–on transitions of blinking quantum dots

F Gao, P Bajwa, A Nguyen, CD Heyes - ACS nano, 2017 - ACS Publications
The majority of quantum dot (QD) blinking studies have used a model of switching between
two distinct fluorescence intensity levels,“on” and “off”. However, a distinct intermediate …

A charge for blinking

TD Krauss, JJ Peterson - Nature materials, 2012 - nature.com
No accepted description of luminescent blinking in quantum dots is currently available. Now,
experiments probing the connection between charge and fluorescence intensity fluctuations …

Modified power law behavior in quantum dot blinking: a novel role for biexcitons and auger ionization

JJ Peterson, DJ Nesbitt - Nano letters, 2009 - ACS Publications
Single photon detection methods are used to acquire fluorescence trajectories from single
CdSe/ZnS colloidal quantum dots (QDs) and analyze their blinking behavior. Although the …

Blinking Suppression in CdSe/ZnS Single Quantum Dots by TiO2 Nanoparticles

M Hamada, S Nakanishi, T Itoh, M Ishikawa, V Biju - ACS nano, 2010 - ACS Publications
The photoluminescence of semiconductor quantum dots and fluorescence of single
molecules intermittently turn ON and OFF, a phenomenon referred to as blinking. In quantum …

Photoinduced dark fraction due to blinking and photodarkening probability in aqueous CdTe quantum dots

AVR Murthy, P Patil, S Datta, S Patil - The Journal of Physical …, 2013 - ACS Publications
We provide a novel approach to measure the photoinduced dark fraction due to blinking in
semiconductor quantum dots in dilute aqueous solution using fluorescence correlation …

Robustness of quantum dot power-law blinking

P Bharadwaj, L Novotny - Nano letters, 2011 - ACS Publications
Photon emission from quantum dots (QDs) and other quantum emitters is characterized by
abrupt jumps between an “on” and an “off” state. In contrast to ions and atoms however, the …

Effect of the shell on the blinking statistics of core-shell quantum dots: A single-particle fluorescence study

CD Heyes, AY Kobitski, VV Breus, GU Nienhaus - Physical Review B …, 2007 - APS
Fluorescence blinking of single quantum dots (QDs) under constant illumination has
attracted a great deal of attention from both experimentalists and theoreticians. To explain …

Single molecule studies of quantum dot fluorescence intermittency: Evidence for both dark and light-assisted blinking dynamics

TA Baker, JL Rouge, DJ Nesbitt - Molecular Physics, 2009 - Taylor & Francis
The present work investigates single CdSe QD blinking behaviour in the absence of
illumination, in order to elucidate the role of photoexcitation on the long time dynamics. The …

Direct measurement of off-state trapping rate fluctuations in single quantum dot fluorescence

AA Cordones, TJ Bixby, SR Leone - Nano letters, 2011 - ACS Publications
Fluorescence decay times measured during the off-state of single CdSe/ZnS quantum dot
blinking are found to decrease with increasing off-state duration, contradicting the charging …