Inferring molecular orientations from vibrational sum frequency generation (SFG) spectra is
challenging in polarization combinations that result in low signal intensities, or when the …

We report a numerical algorithm, the maximum entropy method (MEM), to obtain the
absolute phase of the sum frequency signal from vibrational sum frequency generation …

We combine deuterium labeling, density functional theory calculations, and experimental
vibrational sum frequency generation spectroscopy into a form of “counterfactual-enabled …

Many essential processes occur at soft interfaces, from chemical reactions on aqueous
aerosols in the atmosphere to biochemical recognition and binding at the surface of cell …

Vibrational sum-frequency generation (SFG) spectroscopy can provide valuable qualitative
and quantitative information about molecular species at surface and buried interfaces. For …

We present ways in which pulse sequences and polarizations can be used to extract
structural information from one-and two-dimensional vibrational sum frequency generation …

The interface selectivity of vibrational sum frequency generation (VSFG) spectroscopy is
explained under the dipole approximation as resulting from the breakdown of inversion …

Sum-frequency generation (SFG) spectroscopy provides a unique optical probe for
interfacial molecules with interface-specificity and molecular specificity. SFG measurements …

Orientational time correlation functions (TCFs) are derived for vibrational sum-frequency
generation (VSFG) spectroscopy of the symmetric and asymmetric stretches of high …

Sum-frequency generation vibrational spectroscopy (SFG-VS) can provide detailed
information and understanding of the molecular composition, interactions, and orientational …